Comparative Mossbauer and magnetization study of 1% (119)Sn-doped La(0.67)Ca(0.33)MnO(3) and La(0.67)Sr(0.33)MnO(3)

dc.contributor.authorAssaridis, E.en
dc.contributor.authorPanagiotopoulos, I.en
dc.contributor.authorMoukarika, A.en
dc.contributor.authorBakas, T.en
dc.date.accessioned2015-11-24T18:31:33Z
dc.date.available2015-11-24T18:31:33Z
dc.identifier.issn1098-0121-
dc.identifier.urihttps://olympias.lib.uoi.gr/jspui/handle/123456789/16489
dc.rightsDefault Licence-
dc.subjectphase-separationen
dc.subjectferromagnetic manganitesen
dc.subjectmanganese perovskitesen
dc.subjectdoped manganitesen
dc.subjecttransitionen
dc.subjectmagnetoresistanceen
dc.subjectla1-xcaxmno3en
dc.subjectdependenceen
dc.subjectdynamicsen
dc.subjectphysicsen
dc.titleComparative Mossbauer and magnetization study of 1% (119)Sn-doped La(0.67)Ca(0.33)MnO(3) and La(0.67)Sr(0.33)MnO(3)en
heal.abstractA detailed comparative Mossbauer study of La(0.67)Ca(0.33)MnO(3) and La(0.67)Sr(0.33)MnO(3) samples doped with 1% Sn is presented. The spectra at 5 K can be analyzed by a single ferromagnetic component. However, at higher temperatures two separate ferromagnetic components and a paramagnetic one are required to fit the spectra. The ferromagnetic component with the lower hyperfine field is attributed to clusters of weakened double-exchange interactions due to competition by localization mechanisms. Clear differences between the two samples in regard to the critical behavior arise: (i) The hyperfine field of La(0.67)Ca(0.33)Mn(0.99)Sn(0.01)O(3) disappears abruptly at T(c) in contrast to that of La(0.67)Sr(0.33)Mn(0.99)Sn(0.01)O(3) which varies continuously and goes to zero smoothly at the critical temperature. (ii) The second ferromagnetic phase appears above 0.35T(c) in the Ca sample but only above 0.83T(c) in the Sr sample. The paramagnetic component appears for T > 0.67T(c) in the former compared to T > 0.9T(c) in the latter. The results support recent studies that show differences in the polaronic character, and critical behavior thereof, between the two materials.en
heal.accesscampus-
heal.fullTextAvailabilityTRUE-
heal.identifier.primaryDoi 10.1103/Physrevb.75.224412-
heal.identifier.secondary<Go to ISI>://000247624800059-
heal.identifier.secondaryhttp://prb.aps.org/abstract/PRB/v75/i22/e224412-
heal.journalNamePhysical Review Ben
heal.journalTypepeer reviewed-
heal.languageen-
heal.publicationDate2007-
heal.recordProviderΠανεπιστήμιο Ιωαννίνων. Σχολή Επιστημών και Τεχνολογιών. Τμήμα Βιολογικών Εφαρμογών και Τεχνολογιώνel
heal.typejournalArticle-
heal.type.elΆρθρο Περιοδικούel
heal.type.enJournal articleen

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