Single photon-induced symmetry breaking of H-2 dissociation

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dc.contributor.authorMartin, F.en
dc.contributor.authorFernandez, J.en
dc.contributor.authorHavermeier, T.en
dc.contributor.authorFoucar, L.en
dc.contributor.authorWeber, T.en
dc.contributor.authorKreidi, K.en
dc.contributor.authorSchoffler, M.en
dc.contributor.authorSchmidt, L.en
dc.contributor.authorJahnke, T.en
dc.contributor.authorJagutzki, O.en
dc.contributor.authorCzasch, A.en
dc.contributor.authorBenis, E. P.en
dc.contributor.authorOsipov, T.en
dc.contributor.authorLanders, A. L.en
dc.contributor.authorBelkacem, A.en
dc.contributor.authorPrior, M. H.en
dc.contributor.authorSchmidt-Bocking, H.en
dc.contributor.authorCocke, C. L.en
dc.contributor.authorDorner, R.en
dc.date.accessioned2015-11-24T18:35:27Z
dc.date.available2015-11-24T18:35:27Z
dc.identifier.issn0036-8075-
dc.identifier.urihttps://olympias.lib.uoi.gr/jspui/handle/123456789/17098
dc.rightsDefault Licence-
dc.subjectphotoelectron angular-distributionsen
dc.subjecthydrogen moleculeen
dc.subjectb-splinesen
dc.subjectphotoionizationen
dc.subjectstatesen
dc.subjectlocalizationen
dc.subjectionizationen
dc.subjectelectronsen
dc.subjectregionen
dc.subjectd-2en
dc.titleSingle photon-induced symmetry breaking of H-2 dissociationen
heal.abstractH-2, the smallest and most abundant molecule in the universe, has a perfectly symmetric ground state. What does it take to break this symmetry? We found that the inversion symmetry can be broken by absorption of a linearly polarized photon, which itself has inversion symmetry. In particular, the emission of a photoelectron with subsequent dissociation of the remaining H-2(+) fragment shows no symmetry with respect to the ionic H+ and neutral H atomic fragments. This lack of symmetry results from the entanglement between symmetric and antisymmetric H-2(+) states that is caused by autoionization. The mechanisms behind this symmetry breaking are general for all molecules.en
heal.accesscampus-
heal.fullTextAvailabilityTRUE-
heal.identifier.primaryDOI 10.1126/science.1136598-
heal.identifier.secondary<Go to ISI>://000243909400038-
heal.identifier.secondaryhttp://www.sciencemag.org/content/315/5812/629-
heal.journalNameScienceen
heal.journalTypepeer reviewed-
heal.languageen-
heal.publicationDate2007-
heal.recordProviderΠανεπιστήμιο Ιωαννίνων. Σχολή Επιστημών και Τεχνολογιών. Τμήμα Βιολογικών Εφαρμογών και Τεχνολογιώνel
heal.typejournalArticle-
heal.type.elΆρθρο Περιοδικούel
heal.type.enJournal articleen

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